![]() 4 The studies of the exchange interaction between the triplet excited state and radical spin(s) will give very important knowledge on the forthcoming excited-state organic spintronics and photocontrol of the magnetic properties. However, most of these studies are limited to ground-state systems. 3 Intra- or intermolecular spin alignment and exchange interaction through π-conjugation or π-orbital packing in purely organic spin systems play key roles in their research fields. Π-Radicals have become quite important research targets for organic spintronics 1 as well as molecular-based magnetism, 2 since a large negative magneto-resistance of organic radical system was demonstrated by Sugawara et al.
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